Research Article

Predicting Radiative Heat Transfer in Oxy-Methane Flame Simulations: An Examination of Its Sensitivities to Chemistry and Radiative Property Models

Table 1

A summary of previous CFD studies of oxy-methane/natural gas combustion.

ReferenceSystemChemistry modelsRadiation modelingResults and conclusions

Prieler et al. [24]Turbulent high temperature furnace for smelting and annealing applicationsEddy dissipation concept (EDC) with 46 reversible reactions, steady laminar flamelet (SFM) approach with flamelet libraries generated employing 25-step, 46-step mechanisms as well as 325 reactions in GRI-Mech 3.0Default WSGGM in ANSYS FLUENT (gray model) employed with P-1 and discrete ordinates (DO) radiation modelsTemperature and species concentration predictions from EDC and SFM were very similar. SFM calculations were about 5 times faster than the EDC calculations that employed detailed chemistry. The P1 radiation model overestimated emission and predicted lower temperatures than measurements

Nemitallah and Habib [25]Turbulent, diffusion flame in a gas-turbine combustor investigated for a wide range of operational parametersModified 2-step chemistry mechanism [16]DO radiation model; radiative property model was not specifiedOverall flame shape and exhaust gas concentrations were well-predicted employing the modified two-step mechanisms

Galletti et al. [26]3 MW semi-industrial burnerEddy dissipation model (EDM), EDC, modified global mechanismsP1/DO, revised WSGGM coefficients [10]Turbulence chemistry interactions play an important role in determining the temperature and species concentrations; EDC provides satisfactory temperature and species predictions

Wheaton et al. [27]0.8 MW turbulent burner, high temperature air combustion (HTAC) burnerNonadiabatic equilibrium PDFDO radiation model, revised WSGGM [28] employed in nongray simulationsReasonable agreement of temperature with measurements, high concentrations of radiatively participating gases by themselves are not enough to warrant the use of nongray models. The peak temperatures, temperature gradients, and furnace dimensions also need to be taken into consideration

Yin et al. [17]Semi-industrial furnaceGlobal 2-step and 4-step reaction mechanisms [14, 15] as well as modified versions of these mechanismsDO radiation model, revised WSGGM [11] employed in gray simulationsThe refined chemistry models were able to better predict the temperature and CO concentrations downstream of the furnace

Bhadraiah and Raghavan [29]Laminar, unconfinedFour global mechanisms, 43-step skeletal mechanismOptically thin radiation modelMajor gases and temperature predictions from the 2-step are closer to the 43-step mechanism. Two-step mechanism predicts the location of the reaction zone accurately. Improvements agree at higher flow rates but only qualitative prediction of CO

Kim et al. [30]0.78 MW turbulent natural gas furnaceConservative conditional moment closure for turbulence chemistry interactions with detailed chemistry mechanismsRadiation model and the determination of radiative properties not specifiedA good qualitative agreement is obtained with the temperature overestimated at short radial distances. CO2 was underestimated and CO was overestimated in the high temperature regions

Bennett et al. [31]Laminar, unconfined diffusion flamesGRI-Mech 3.0Optically thin radiation modelComputational and experimental flame lengths and maximum centerline temperatures show excellent agreement. Radial profiles when plotted at fixed values of a dimensionless axial coordinate also show excellent agreement

Abdul-Sater and Krishnamoorthy [21]Laminar, confined diffusion flamesNonadiabatic equilibrium PDFDO radiation model, revised WSGGM [28] employed in gray and nongray simulationsComputational and experimental flame lengths and temperature profiles show excellent agreement. Significant variations in the flame radiant fraction predictions between the gray and nongray models